| | First Man (2008) (pre-production) .... Business Mogul/First Man |
| | Frankie Machine (2008) (pre-production) (attached) .... Frankie Machine |
| | Sugarland (2008) (pre-production) .... Alfy Fanjul |
| | Heat (2007) (VG) (pre-production) (in negotiations) .... Neil McCauley |
| | Righteous Kill (2008) (filming) |
| | What Just Happened? (2008) (post-production) .... Ben |
| | Stardust (2007) .... Captain Shakespeare |
| | The Good Shepherd (2006) .... Bill Sullivan |
| | Arthur and the Invisibles (2006) (voice: English version) .... King |
| | Hide and Seek (2005) .... David Callaway |
| | The Bridge of San Luis Rey (2004) .... Archbishop of Peru |
| | Meet the Fockers (2004) .... Jack Byrnes |
| | Shark Tale (2004) (voice) .... Don Lino |
| | Godsend (2004) .... Richard Wells |
| | Analyze That (2002) .... Paul Vitti |
| | City by the Sea (2002) .... Vincent LaMarca |
| | Showtime (2002) .... Det. Mitch Preston |
| | The Score (2001) .... Nick Wells |
| | 15 Minutes (2001) .... Detective Eddie Flemming |
| | Meet the Parents (2000) .... Jack Byrnes |
| | Men of Honor (2000) .... Chief Leslie W. 'Billy' Sunday |
| | The Adventures of Rocky & Bullwinkle (2000) .... Fearless Leader |
| | Flawless (1999) .... Walt Koontz |
| | Analyze This (1999) .... Paul Vitti |
| | Ronin (1998) .... Sam |
| | Great Expectations (1998) .... Arthur Lustig |
| | Jackie Brown (1997) .... Louis Gara |
| | Wag the Dog (1997) .... Conrad Brean |
| | Cop Land (1997) .... Lt. Moe Tilden |
| | Marvin's Room (1996) .... Dr. Wally |
| | Sleepers (1996) .... Father Bobby |
| | The Fan (1996) .... Gil Renard |
| | Heat (1995) .... Neil McCauley |
| | Casino (1995) .... Sam 'Ace' Rothstein |
| | Cent et une nuits de Simon Cinéma, Les (1995) .... Le mari de la star-fantasme en croisière |
| | Frankenstein (1994) .... The Creature |
| | ... aka Mary Shelley's Frankenstein |
| | A Bronx Tale (1993) .... Lorenzo Anello |
| | This Boy's Life (1993) .... Dwight Hansen |
| | Mad Dog and Glory (1993) .... Wayne 'Mad Dog' Dobie |
| | Night and the City (1992) .... Harry Fabian |
| | Mistress (1992) .... Evan M. Wright |
| | The Godfather Trilogy: 1901-1980 (1992) (V) .... Young Don Vito Corleone |
| | Cape Fear (1991) .... Max Cady |
| | Backdraft (1991) .... Donald 'Shadow' Rimgale |
| | Guilty by Suspicion (1991) .... David Merrill |
| | Awakenings (1990) .... Leonard Lowe |
| | Goodfellas (1990) .... Jimmy Conway |
| | Stanley & Iris (1990) .... Stanley Everett Cox |
| | We're No Angels (1989) .... Ned |
| | Jacknife (1989) .... Joseph 'Jacknife' Megessey |
| | Midnight Run (1988) .... Jack Walsh |
| | The Untouchables (1987) .... Al Capone |
| | Angel Heart (1987) .... Louis Cyphre |
| | The Mission (1986) .... Rodrigo Mendoza |
| | Brazil (1985) .... Archibald 'Harry' Tuttle |
| | Falling in Love (1984) .... Frank Raftis |
| | Once Upon a Time in America (1984) .... David 'Noodles' Aaronson |
| | The King of Comedy (1983) .... Rupert Pupkin |
| | True Confessions (1981) .... Des Spellacy |
| | Raging Bull (1980) .... Jake La Motta |
| | The Deer Hunter (1978) .... Michael Vronsky |
| | "The Godfather Saga" (1977) (mini) TV Series .... Young Vito Corleone |
| | New York, New York (1977) .... Jimmy Doyle |
| | The Last Tycoon (1976) .... Monroe Stahr |
| | Novecento (1976) .... Alfredo Berlinghieri |
| | Taxi Driver (1976) (as Robert DeNiro) .... Travis Bickle |
| | The Godfather: Part II (1974) .... Vito Corleone |
| | Mean Streets (1973) .... John 'Johnny Boy' Civello |
| | Bang the Drum Slowly (1973) .... Bruce Pearson |
| | The Gang That Couldn't Shoot Straight (1971) .... Mario |
| | Born to Win (1971) .... Danny |
| | Jennifer on My Mind (1971) .... Mardigian |
| | Hi, Mom! (1970) .... Jon Rubin |
| | Bloody Mama (1970) .... Lloyd Barker |
| | The Wedding Party (1969) .... Cecil |
| | Sam's Song (1969) .... Sam Nicoletti |
| | Greetings (1968) .... Jon Rubin |
| | Trois chambres à Manhattan (1965) (uncredited) .... Client at the diner... aka Three Rooms in Manhattan (International: English title) |